Next-generation toys are designed to entertain and interact with children. Such toys need a power source, generally a battery that must be replaced frequently, leading to increased maintenance costs. Recently, an innovative biomechanical energy harvester called a triboelectric nanogenerator (TENG) was introduced as an eco-friendly generator that scavenges waste energy. Here, in a step toward the commercialization of TENG devices, we present a novel approach that uses TENG technology to develop battery-free electronic smart toys. This robust, eco-friendly, and cost-effective approach for harnessing biomechanical energy can transform a traditional toy into a smart toy. With this innovative idea, we developed a smart clapping toy (SCT-TENG) and a smart duck toy (SDT-TENG) using biocompatible materials. We employed a simple inbuilt circuit with light-emitting diodes that are powered using biomechanical energy. The SCT-TENG and SDT-TENG exhibited output voltages of 65 Vp-p and 260 Vp-p, respectively. We believe that the use of TENG technology for battery-free electronic smart toys opens up new possibilities for the commercialization of TENGs and the field of battery-free smart toys. © 2018 American Chemical Society.